Structure and properties of NdCuGa3 single crystals

Binod K. Rai, Boris Maiorov, Krzysztof Gofryk, Patrick O'Rourke, Catherine Housley, Henry Ajo, Asraf Sawon, Arjun K. Pathak, Narayan Poudel, Qiang Zhang, Travis J. Williams, Matthias Frontzek

Research output: Contribution to journalArticlepeer-review

1 Scopus citations

Abstract

This manuscript reports on the structural and magnetic properties of NdCuGa3 using powder and single crystal X-ray diffraction (XRD), zero-field single crystal neutron diffraction, magnetization, and specific heat measurements. Our XRD on a single crystal specimen of NdCuGa3 confirmed that it crystallizes in the tetragonal BaNiSi3-type structure. A magnetic phase transition at TN= 3.3 K is assessed using specific heat and ac magnetic susceptibility measurements. No additional anomaly below TN down to 50 mK was detected by performing specific heat measurements. Neutron single crystal diffraction data collected at T= 300 mK confirm the antiferromagnetic phase below TN= 3.3 K with the propagation vector τ→= (0.2, 0, 0). Possible magnetic structure solutions of NdCuGa3 are discussed.

Original languageEnglish
Article number171515
JournalJournal of Magnetism and Magnetic Materials
Volume589
Early online dateNov 19 2023
DOIs
StatePublished - Jan 1 2024

Keywords

  • Antiferromagnetism
  • Crystal structure
  • Flux growth
  • Neutron diffraction
  • Specific heat
  • X-ray diffraction

INL Publication Number

  • INL/JOU-24-79943
  • 182850

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